Maider Junkal Echeveste Medrano

57 Sulfide toxicity as key control on anaerobic oxidation of methane in eutrophic coastal sediments Figure 2. Porewater depth profiles of sulfate (SO4 2–), methane (CH4), sulfide (H2S), dissolved iron (Fe2+) and manganese (Mn2+/3+), ammonium (NH4 +) and the sum of nitrate and nitrite (NO x) at our study sites in the Stockholm Archipelago: Site 3 (Sandofjärden), Site 5 (Lilla Värtan) and Site 7 (Skurusundet). The arrow to the left indicates decreasing bottom water (BW) oxygen concentrations from Site 3 to 7. Cmbsf; centimeters below the seafloor. The calculated downward flux of sulfate into the SMTZ (Table 3) was highest at Sites 5 and 7 (1.5 and 1.3 mmol m-2 d-1), but still substantial (0.9 mmol m-2 d-1) at Site 3. The calculated upward flux of methane into the SMTZ at Site 3 was nearly absent, and around 0.5 mmol m-2 d-1 at Sites 5 and 7, which should be regarded as an absolute minimum estimate due to degassing of methane during sampling (Egger et al., 2016; Melaniuk et al., 2022). There was no benthic methane efflux at Site 3. The benthic methane efflux was about seven times larger at Site 7 relative to Site 5 (~ 1 vs. 0.15 mmol m-2 d-1, respectively). 2

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